Replication Data for: "Strain in Halide Perovskites and Solar Cell Stability: Accelerated Stress Tests under Bias Voltage".

DOI

The lifespan of halide perovskite solar cells (PSCs) is currently a major concern for the implementation and commercialization of the technology. Tensile and compressive strain alters the halide perovskite (HP) lattice under operando conditions, affecting PSC stability. However, the mechanisms governing strain responses are still unknown. In this work, we monitored the evolution of strain in PSCs during accelerated stability tests under continuous light irradiation and bias-voltage. Additive engineering led to the compression of the HP lattice improved PSC stability. The temporal evolution of the HP lattice, together with the electrical response of devices employing modified and reference HP, were tracked by in-situ X-ray diffraction, photoluminescence, and quasi in-situ electrochemical impedance spectroscopy. Our results demonstrate a good correlation between lattice expansion (strain) with the device’s current decay and stability. Additionally, and contrary to current understanding, we observed that lattice compression in HP was not sufficient to ensure protection against degradation.

Identifier
DOI https://doi.org/10.34810/data1898
Related Identifier IsCitedBy https://doi.org/10.1021/acsenergylett.4c02822
Metadata Access https://dataverse.csuc.cat/oai?verb=GetRecord&metadataPrefix=oai_datacite&identifier=doi:10.34810/data1898
Provenance
Creator Baumann, Fanny ORCID logo; Karimipour, Masoud ORCID logo; Ruiz Raga, Sonia ORCID logo; Padilla-Pantoja, Jessica ORCID logo; Caicedo Roque, Jose Manuel ORCID logo; Chávez-Ángel, Emigdio ORCID logo; Alcalá Ibarra, Alex ORCID logo; Rémy Pouteaux; Santiso, Jose ORCID logo; Lira-Cantu, Monica ORCID logo
Publisher CORA.Repositori de Dades de Recerca
Contributor Baumann, Fanny; Ruiz Raga, Sonia; Institut Català de Nanociència i Nanotecnologia
Publication Year 2025
Rights CC BY 4.0; info:eu-repo/semantics/openAccess; http://creativecommons.org/licenses/by/4.0
OpenAccess true
Contact Baumann, Fanny (ICN2); Ruiz Raga, Sonia (ICN2)
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Version 1.1
Discipline Chemistry; Construction Engineering and Architecture; Earth and Environmental Science; Engineering; Engineering Sciences; Environmental Research; Geosciences; Natural Sciences; Physics