Further investigation of the methanol to gasoline reaction over ZSM-5 using INS

DOI

The reaction of methanol to form hydrocarbons over zeolite catalysts is an important option for conversion of natural gas or coal to liquid fuels. We have shown previously (RB1610409, April 2016, RB1620416, September 2016) that INS can observe the hydrocarbon species present in the pores of a working commercial catalyst. In this project we wish to better understand the chemistry leading to deactivation of the catalyst by looking at catalysts which are partially or completely deactivated after long periods of reaction. To help in interpret the spectra obtained in earlier experiments and in the proposed experiments we will also measure spectra from model compounds adsorbed in the zeolite. The experiments are proposed for the MAPS spectrometer which has the highest available resolution over the energy range of interest (400-4000 cm-1).

Identifier
DOI https://doi.org/10.5286/ISIS.E.84806126
Metadata Access https://icatisis.esc.rl.ac.uk/oaipmh/request?verb=GetRecord&metadataPrefix=oai_datacite&identifier=oai:icatisis.esc.rl.ac.uk:inv/84806126
Provenance
Creator Ms Andrea Zachariou; Dr Alexander Hawkins; Dr Santhosh Matam; Professor Russell Howe; Professor Stewart Parker; Professor David Lennon; Professor Richard Catlow; Dr Antok Suwardiyanto; Dr Paul Collier; Dr James McGregor
Publisher ISIS Neutron and Muon Source
Publication Year 2021
Rights CC-BY Attribution 4.0 International; https://creativecommons.org/licenses/by/4.0/
OpenAccess true
Contact isisdata(at)stfc.ac.uk
Representation
Resource Type Dataset
Discipline Chemistry; Natural Sciences
Temporal Coverage Begin 2017-03-10T09:19:55Z
Temporal Coverage End 2018-12-09T08:17:00Z