Crystalline electric field levels in a rare-earth triangular-lattice antiferromagnet

DOI

Rare-earth frustrated systems can present exotic physical properties. The newly discovered TmMgGaO4 shares the same structure as the quantum spin liquid candidate YbMgGaO4 with layered triangular lattice. Due to strong spin orbital coupling and crystalline electric field, its ground state is a singlet, a non-Kramers doublet or a quasi-doublet composed of two singlets. Different ground states will have different spin Hamiltonians. For example, Ising spin state has been proposed for the quasi-doublet scenario which, however, is inconsistent with the susceptibility measurement. Here we propose to use inelastic neutron scattering to study the crystalline field of TmMgGaO4 so that the ground state can be determined which can help us decide the spin Hamiltonian.

Identifier
DOI https://doi.org/10.5286/ISIS.E.98001182
Metadata Access https://icatisis.esc.rl.ac.uk/oaipmh/request?verb=GetRecord&metadataPrefix=oai_datacite&identifier=oai:icatisis.esc.rl.ac.uk:inv/98001182
Provenance
Creator Mr Jun Zhao; Dr Helen Walker; Mr Yao Shen
Publisher ISIS Neutron and Muon Source
Publication Year 2021
Rights CC-BY Attribution 4.0 International; https://creativecommons.org/licenses/by/4.0/
OpenAccess true
Contact isisdata(at)stfc.ac.uk
Representation
Resource Type Dataset
Discipline Natural Sciences; Physics
Temporal Coverage Begin 2018-10-03T08:00:00Z
Temporal Coverage End 2018-10-05T08:34:25Z