Understanding the Li conduction path and corrosion processes on Li7-3xGaxLa3Zr2O12 garnet electrolytes

DOI

Recently we have developed a family of fast Li-conducting garnets via doping with Li7-3xGaxLa3Zr2O12 (0 ≤ x ≤ 0.5) system. The measured bulk conductivities at room temperature are >10-3 S/cm, at least one order of magnitude higher than currently reported materials (unprecedented, to the best of our knowledge as of September 2013), and approaching liquid electrolyte conductivity values. DFT simulations, in-house NMR and microstructural measurements support successful Ga-incorporation into the garnet structure, but the interplay between Ga, Li and proton distributions is crucial to understand this high conductivity. Moreover the corrosion process with moisture need to be understand in this materials for processing purpose and integration into devices. For this purpose we ask for 3 days at HRPD to measure 8 samples at RT under different ageing processes

Identifier
DOI https://doi.org/10.5286/ISIS.E.59894632
Metadata Access https://icatisis.esc.rl.ac.uk/oaipmh/request?verb=GetRecord&metadataPrefix=oai_datacite&identifier=oai:icatisis.esc.rl.ac.uk:inv/59894632
Provenance
Creator Dr Carlos Bernuy; Professor John Kilner; Mr William Manalastas; Dr Fred Aguesse; Dr Ainara Aguadero; Dr Kevin Knight
Publisher ISIS Neutron and Muon Source
Publication Year 2017
Rights CC-BY Attribution 4.0 International; https://creativecommons.org/licenses/by/4.0/
OpenAccess true
Contact isisdata(at)stfc.ac.uk
Representation
Resource Type Dataset
Discipline Photon- and Neutron Geosciences
Temporal Coverage Begin 2014-06-25T23:00:00Z
Temporal Coverage End 2014-06-26T23:00:00Z