Phonon lifetimes of the thermoelectric material sodium cobaltate

DOI

Sodium cobaltate has excellent thermoelectric properties, including low thermal conductivity. We have measured its phonon dispersion using inelastic x-ray scattering, and we find that it has well defined modes unlike a phonon glass. First-principles density-functional calculations are in excellent agreement with the data, and we identify a rattling mode. We now propose to use the better energy resolution of inelastic neutron scattering on IN8 to measure the energy line widths of selected modes as a function of temperature. This will allow us to determine the phonon lifetimes and estimate the lattice contribution to the thermal conductivity.

Identifier
DOI https://doi.org/10.5291/ILL-DATA.7-01-369
Metadata Access https://data.ill.fr/openaire/oai?verb=GetRecord&metadataPrefix=oai_datacite&identifier=10.5291/ILL-DATA.7-01-369
Provenance
Creator Piovano, Andrea; Voneshen, David; Goff, Jonathan; Refson, Keith; Enderle, Mechthild
Publisher Institut Laue-Langevin
Publication Year 2014
Rights OpenAccess; info:eu-repo/semantics/openAccess
OpenAccess true
Representation
Resource Type Dataset
Size 5 MB
Version 1
Discipline Particles, Nuclei and Fields