Null Isotope Study of Lithium Borogermanate Glasses

DOI

Alkali borogermanate glasses are topologically complex, in that [BOn] (n = 3, 4)and [GeOn] (n = 4, 5, 6) polyhedra may all coexist. Equilibrium between these structural units has significant influence on physico-chemical properties such as conductivity and corrosion resistance. In previous work on the potassium system we used neutron diffraction and NMR to show that K preferentially associates with borate units to form [BO4] in preference to [GeO5] or [GeO6], giving an increase in average coordination of B from 3 to 3.8 but of Ge from 4 to only 4.3. We wish to repeat the study with the lithium system where we can take advantage of the opposite signs of the scattering lengths of the Li-6 and Li-7 isotopes to produce samples which show null scattering from Li. This simplifies the problem and, by comparison with samples formed with natural Li we can study the Li environment itself.

Identifier
DOI https://doi.org/10.5286/ISIS.E.58447316
Metadata Access https://icatisis.esc.rl.ac.uk/oaipmh/request?verb=GetRecord&metadataPrefix=oai_datacite&identifier=oai:icatisis.esc.rl.ac.uk:inv/58447316
Provenance
Creator Dr Oliver Alderman; Mr Faizani Mohd Noor; Dr Diane Holland; Dr Alex Hannon
Publisher ISIS Neutron and Muon Source
Publication Year 2018
Rights CC-BY Attribution 4.0 International; https://creativecommons.org/licenses/by/4.0/
OpenAccess true
Contact isisdata(at)stfc.ac.uk
Representation
Resource Type Dataset
Discipline Photon- and Neutron Geosciences
Temporal Coverage Begin 2015-04-20T00:00:00Z
Temporal Coverage End 2015-06-18T14:11:30Z