Exploring nanoscale phase separation in alpha-NaMnO2 and CuMnO2 2D frustrated antiferromagnets by atomic PDF analysis

DOI

Recently, our combined diffraction and NMR experiments have shown that alpha-NaMnO2, an antiferromagnet with two-dimensional triangular stacked topology, is a striking example of an insulating system where the spin, degree of freedom induces multiple competing phases. In order to shed light in the role of geometric spin frustration, studies of isostructural compounds by total scattering approaches are highly sought. For this reason we request 5-days of beam time on GEM to raise evidence on the evolution of the near-equivalent structural phases of alpha-NaMnO2 against the case of the isostructural, more homogeneous CuMnO2. By analyzing their atomic pair distribution function (PDF) data, we aim to learn how the competition evolves into locally broken symmetry states when the critical region is approached and the transformation from the disordered to the Néel ordered states takes place.

Identifier
DOI https://doi.org/10.5286/ISIS.E.73941796
Metadata Access https://icatisis.esc.rl.ac.uk/oaipmh/request?verb=GetRecord&metadataPrefix=oai_datacite&identifier=oai:icatisis.esc.rl.ac.uk:inv/73941796
Provenance
Creator Dr Antonio Fernandez-Martinez; Professor David Keen; Dr Alexandros Lappas; Dr Emil Bozin
Publisher ISIS Neutron and Muon Source
Publication Year 2019
Rights CC-BY Attribution 4.0 International; https://creativecommons.org/licenses/by/4.0/
OpenAccess true
Contact isisdata(at)stfc.ac.uk
Representation
Resource Type Dataset
Discipline Natural Sciences; Physics
Temporal Coverage Begin 2016-02-24T08:00:00Z
Temporal Coverage End 2016-02-29T08:00:00Z