Fluorophosphate Derivatives of Gypsum and Lithium in Biogenic Manganese Oxides

DOI

This proposal seeks neutron diffraction beamtime to study two important systems. We have demonstrated that monofluorophosphate (PO3F) can be substituted into gypsum (CaSO4.2H2O) to provide an improved biocement. However, we wish to study the structural implications of the replacement of SO4 by isoelectronic PO3F and the implication on reduced hydrogen bonding to the structural water molecules commonly seen with the presence of fluorine. The second part of this proposal seeks to study lithium manganese oxides formed from biogenic sources. Biogenic Mn oxide is a low cost alternative to synthetic forms and is environmental friendly and can be used to extract lithium for the environment. Indeed, initial results show improved Li uptake with biogenic forms. However the subtle differences in structure have yet to be studied in detail and neutron diffraction offers such an opportunity.

Identifier
DOI https://doi.org/10.5286/ISIS.E.24088662
Metadata Access https://icatisis.esc.rl.ac.uk/oaipmh/request?verb=GetRecord&metadataPrefix=oai_datacite&identifier=oai:icatisis.esc.rl.ac.uk:inv/24088662
Provenance
Creator Dr Adrian Wright; Miss Michaela Yates; Miss Julie Rutter; Dr Annabelle Baker
Publisher ISIS Neutron and Muon Source
Publication Year 2015
Rights CC-BY Attribution 4.0 International; https://creativecommons.org/licenses/by/4.0/
OpenAccess true
Contact isisdata(at)stfc.ac.uk
Representation
Resource Type Dataset
Discipline Photon- and Neutron Geosciences
Temporal Coverage Begin 2012-03-20T09:35:55Z
Temporal Coverage End 2012-03-29T07:51:27Z