The effect of pressure on the hydrogen bonding in ammonium formate

DOI

We propose to investigate the changes that occur in the structure of ammonium formate as a function of pressure. This is the simplest system in which the oxygen atoms of a carboxylate group are hydrogen bonded to the hydrogen atoms of an NH group. This compound is known to undergo a phase transition at 1.8 GPa, during which there is a significant reorganization of the hydrogen-bonding network. We will determine the evolution of the changes within the hydrogen bonds for both phases. In particular the hydrogen bonding in the high pressure phase is such that for on the oxygen atoms the intermolecular bonding occurs within the plane of the carboxylate group whilst for the other oxygen it is at right angles to this plane. This bonding arrangement gives us an opportunity to investigate the effect of pressure on a system where both in and out of plane hydrogen bonding occurs.

Identifier
DOI https://doi.org/10.5286/ISIS.E.73945894
Metadata Access https://icatisis.esc.rl.ac.uk/oaipmh/request?verb=GetRecord&metadataPrefix=oai_datacite&identifier=oai:icatisis.esc.rl.ac.uk:inv/73945894
Provenance
Creator Dr Craig Bull; Dr Richard Jones; Professor Colin Pulham; Dr Richard Darton
Publisher ISIS Neutron and Muon Source
Publication Year 2019
Rights CC-BY Attribution 4.0 International; https://creativecommons.org/licenses/by/4.0/
OpenAccess true
Contact isisdata(at)stfc.ac.uk
Representation
Resource Type Dataset
Discipline Chemistry; Natural Sciences
Temporal Coverage Begin 2016-03-11T10:00:00Z
Temporal Coverage End 2016-03-14T10:00:00Z