Controlling the morphology of fullerene-free polymer solar cells using additives: a SANS study

DOI

We have recently demonstrated, using small angle neutron scattering in combination with other techniques, that in organic photovoltaic devices (OPVs) the additive 1,8-diiodooctane (DIO) largely remains in the film after spin-coating acting as a plasticizer to increase molecular mobility and allowing morphological improvement of the film with a consequent increase in power conversion efficiency (PCE) of the OPV device. This new finding opens new perspectives into the morphology control of OPVs, namely through the use of additives and mixtures of additives possessing different affinities towards the polymer and the acceptor which will allow us to optimize the corresponding morphology and PCE. In this proposal we plan to use this strategy to improve the morphology and PCE of fullerene-free solar cells based on the high efficient system PBDB-T:ITIC which has a reported PCE > 12%.

Identifier
DOI https://doi.org/10.5286/ISIS.E.87842077
Metadata Access https://icatisis.esc.rl.ac.uk/oaipmh/request?verb=GetRecord&metadataPrefix=oai_datacite&identifier=oai:icatisis.esc.rl.ac.uk:inv/87842077
Provenance
Creator Dr Gabriel Perez Garcia; Dr Hugo Gaspar; Dr Steve King; Professor Richard Jones; Dr Gabriel Bernardo; Dr Andrew Parnell
Publisher ISIS Neutron and Muon Source
Publication Year 2021
Rights CC-BY Attribution 4.0 International; https://creativecommons.org/licenses/by/4.0/
OpenAccess true
Contact isisdata(at)stfc.ac.uk
Representation
Resource Type Dataset
Discipline Photon- and Neutron Geosciences
Temporal Coverage Begin 2018-02-25T00:00:00Z
Temporal Coverage End 2018-10-26T10:19:38Z