D2O Vapour Diffusion at the Air Water Interface

DOI

A theoretical estimate of the H/D exchange rate for an open trough (e.g. D2O in ambient atmosphere, 50% relative humidity) yields an amount of exchanged liquid of the order of 10^-2 g after 800 minutes for a standard ISIS trough. Recent pilot experiments however show a much greater volume exchange (~10g/800 minutes). We would like to perform a quantitative study of H/D exchange at the air-water interface to determine the rates of exchange of D2O vapour into null-reflecting water for different conditions (surface-to-volume, humidity). Furthermore we intend to study the potential formation of a D2O rich layer at the vapour/liquid interface.We expect that the results will help with future planning of reflectivity experiments involving large are open troughs and will reduce the potential for misinterpretation of data. It will also help further the understanding of this fundamental process.

Identifier
DOI https://doi.org/10.5286/ISIS.E.58451436
Metadata Access https://icatisis.esc.rl.ac.uk/oaipmh/request?verb=GetRecord&metadataPrefix=oai_datacite&identifier=oai:icatisis.esc.rl.ac.uk:inv/58451436
Provenance
Creator Dr Luke Clifton; Dr Maxmilian Skoda
Publisher ISIS Neutron and Muon Source
Publication Year 2018
Rights CC-BY Attribution 4.0 International; https://creativecommons.org/licenses/by/4.0/
OpenAccess true
Contact isisdata(at)stfc.ac.uk
Representation
Resource Type Dataset
Discipline Chemistry; Natural Sciences; Physics
Temporal Coverage Begin 2015-04-13T08:00:00Z
Temporal Coverage End 2015-04-15T08:00:00Z