High-Temperature Neutron Diffraction of Thermoelectric Materials

DOI

We wish to investigate the origin of the promising thermoelectic performance of oxy-chalcogenides BiOCuQ (Q = S, Se, Te) and related phases. We wish to explore whether the low thermal conductivity of these materials at elevated temperatures is related to increasing levels of disorder of copper ions within a PbO-type [Cu2Q2]2- layer. We seek to collect powder neutron diffraction data on the stoichiometric phases in the temperature range 298<T/K<673, to investigate the evolution with temperature of the detailed structure of the Cu2Q2 layer. We also aim to collect data on the first members of a series in which there is partial replacement of trivalent bismuth with divalent lead to investigate the structural impact of the oxidation of copper that results from substitution. We will also collect reference data on Cu2-xSe which has recently been shown to exhibit a high TE figure of merit.

Identifier
DOI https://doi.org/10.5286/ISIS.E.24090143
Metadata Access https://icatisis.esc.rl.ac.uk/oaipmh/request?verb=GetRecord&metadataPrefix=oai_datacite&identifier=oai:icatisis.esc.rl.ac.uk:inv/24090143
Provenance
Creator Professor Anthony Powell; Dr Paz Vaqueiro-Rodriguez; Dr Jan-Willem Bos; Mr Son Luu
Publisher ISIS Neutron and Muon Source
Publication Year 2016
Rights CC-BY Attribution 4.0 International; https://creativecommons.org/licenses/by/4.0/
OpenAccess true
Contact isisdata(at)stfc.ac.uk
Representation
Resource Type Dataset
Discipline Photon- and Neutron Geosciences
Temporal Coverage Begin 2013-02-22T09:12:37Z
Temporal Coverage End 2013-02-25T09:30:29Z