Stability of Shielded Pentacenes under Ambient Conditions [data]

DOI

The stabilization of pentacene through variation of substituents serves as a test bed to access stable organic semiconductors, transferable to the larger soluble acenes and azaacenes. Pentacene is stable enough for derivatization via wet-chemistry but sufficiently labile to test its (induced) (photo)decomposition. In this article, we describe the synthesis of shielded pentacenes, either via covalent jacketing with ester macrocycles or via steric shielding with biphenylyl substituents, together with attempts to access a bis(ortho-quaterphenyl) substituted Geländer pentacene. The photostability of the pentacenes is assessed under ambient conditions (air, light) to simulate handling under typical laboratory conditions and put into perspective with reference compounds, such as TIPS-ethynylated, ether-jacketed or our previously reported Geländer pentacenes.

Identifier
DOI https://doi.org/10.11588/data/HNLJI7
Related Identifier IsCitedBy https://doi.org/10.1002/hlca.202400161
Metadata Access https://heidata.uni-heidelberg.de/oai?verb=GetRecord&metadataPrefix=oai_datacite&identifier=doi:10.11588/data/HNLJI7
Provenance
Creator Ludwig, Philipp ORCID logo; Kilian, Paul; Mayerhofer, Patrick; Hippchen, Nikolai; Rominger, Frank; Freudenberg, Jan (ORCID: 0000-0003-0998-693X); Bunz, Uwe H. F. ORCID logo
Publisher heiDATA
Contributor Ludwig, Philipp; Bunz, Uwe H. F.
Publication Year 2024
Funding Reference Deutsche Forschungsgemeinschaft (SFB) 1249 ; Deutsche Forschungsgemeinschaft INST 40/575-1 FUGG ; Deutsche Forschungsgemeinschaft INST 35/1596-1 FUGG
Rights CC BY 4.0; info:eu-repo/semantics/openAccess; http://creativecommons.org/licenses/by/4.0
OpenAccess true
Contact Ludwig, Philipp (Heidelberg University, OCI); Bunz, Uwe H. F. (Heidelberg University, OCI)
Representation
Resource Type Dataset
Format application/zip; text/plain
Size 4943041; 2788476; 40415415; 352970; 7795183; 586915; 326; 198016; 64065
Version 1.1
Discipline Chemistry; Natural Sciences