A study on how moderate heating renders 7.8 million-year-old organic matter bioavailable in deep marine sediments

DOI

In laboratory experiments on field-collected sediments, we investigated 7.8 million-year-old sediment from a site off the Nankai Trough, Japan, through incubation experiments to simulate future burial conditions. In a 55-day laboratory experiment, we incubated sediment slurried with artificial seawater in four subsets at 20°C (control), and at 35°C, 55°C, and 85°C to simulate future heating during burial and conditions favorable for mesophilic, thermophilic, and hyperthermophilic microorganisms, respectively. We investigated changes in dissolved organic matter quality as a function of microbial activity and temperature using 3D fluorescence spectroscopy (EEMs) and FT-ICR-MS, and analyzed dissolved manganese, iron, and sulfur to detect changes in the sediment's mineral matrix. We observed temperature- and time-dependent changes in the dissolved organic matter (DOM) pool. At 20°C, biotic production of protein-like DOM was predominant, ceasing at higher temperatures. Above 35°C, both protein-like and humic-like DOM were released upon heating, but their reactivity was low. At 55°C, abiotic decomposition of humic compounds led to the generation of protein-like DOM. By 85°C, the DOM composition shifted significantly, with larger molecules rapidly released and nitrogen-containing compounds decomposed, producing H2 and acetate. Data contains (1) bulk parameters about organics and inorganics in the dissolved phase, (2) release of the acetate during laboratory experiments, (3) details about the formulae characterized by Fourier transform ion cyclotron resonance mass spectrometry (FT-ICR-MS).

Identifier
DOI https://doi.pangaea.de/10.1594/PANGAEA.973415
Metadata Access https://ws.pangaea.de/oai/provider?verb=GetRecord&metadataPrefix=datacite4&identifier=oai:pangaea.de:doi:10.1594/PANGAEA.973415
Provenance
Creator Gan, Shuchai ORCID logo; Heuer, Verena B (ORCID: 0000-0002-1856-116X); Adhikari, Rishi Ram ORCID logo; Wörmer, Lars ORCID logo
Publisher PANGAEA
Publication Year 2024
Funding Reference German Research Foundation https://doi.org/10.13039/501100001659 Crossref Funder ID 387745511 https://gepris.dfg.de/gepris/projekt/387745511 Exploring the impact of temperature on dissolved organic matter and life in the deep biosphere off Muroto, Nankai Trough (IODP Expedition 370); German Research Foundation https://doi.org/10.13039/501100001659 Crossref Funder ID 390741603 https://gepris.dfg.de/gepris/projekt/390741603 EXC 2077: The Ocean Floor – Earth's Uncharted Interface
Rights Creative Commons Attribution 4.0 International; Data access is restricted (moratorium, sensitive data, license constraints); https://creativecommons.org/licenses/by/4.0/
OpenAccess false
Representation
Resource Type Bundled Publication of Datasets; Collection
Format application/zip
Size 3 datasets
Discipline Earth System Research
Spatial Coverage (136.917 LON, 32.748 LAT)