C-H and H-H Binding in Coordinatively Unsaturated Ruthenium Carbene Complexes

DOI

Removal of the chloride ligand from the neutral N-heterocyclic carbene complex Ru(IPr)2(CO)HCl (IPr = bis(1,3-(2,6-diisopropylphenyl)imidazol-2-ylidene) by NaBArF4 affords the salt [Ru(IPr)2(CO)H]BArF4 (1), which has been characterised by X-ray crystallography as being stabilised by two agostic Ru...H-C interactions. Addition of an atmosphere of H2 traps this species to afford a spectroscopically characterised dihydrogen hydride complex, [Ru(IPr)2(CO)(eta2-H2)H]BArF4 (2). Neutron data will afford accurate measurement of both Ru...H-C and Ru(eta2-H2)H distances affording structural information crucial to understanding both the stoichiometric and potential catalytic reactivity (e. g. C=C/C=O hydrogenation) of these types of species.

Identifier
DOI https://doi.org/10.5286/ISIS.E.61786765
Metadata Access https://icatisis.esc.rl.ac.uk/oaipmh/request?verb=GetRecord&metadataPrefix=oai_datacite&identifier=oai:icatisis.esc.rl.ac.uk:inv/61786765
Provenance
Creator Dr Mary Mahon; Dr Hazel Sparkes; Professor Michael Whittlesey; Dr Ian Riddlestone; Dr Matthias Gutmann
Publisher ISIS Neutron and Muon Source
Publication Year 2018
Rights CC-BY Attribution 4.0 International; https://creativecommons.org/licenses/by/4.0/
OpenAccess true
Contact isisdata(at)stfc.ac.uk
Representation
Resource Type Dataset
Discipline Chemistry; Natural Sciences
Temporal Coverage Begin 2015-06-25T09:00:00Z
Temporal Coverage End 2015-07-06T09:00:00Z