μXRF and μXANES to unequivocally disclose the nature of the black phases and Hg-Cl and Hg-S-Cl species on blackened Roman cinnabar fresco pa

DOI

The blackening of red cinnabar pigment is a major problem of conservation for the artworks containing it. To explain the black color, different hypotheses have been proposed, but none of them has been fully confirmed. This proposal aims to identify the newly formed black phases, comparing the results in model fresco paintings subjected to accelerated weathering experiments and the ones in blackened cinnabar fresco painting samples from the Archaeological Park of Pompeii. The possible presence of additional Hg-Cl and Hg-S-Cl species, not easily detectable by conventional laboratory techniques, will be also confirmed. The resulting information will allow refining the understanding of the chemical reactivity leading to the darkening of cinnabar, contributing to develop appropriate conservation protocols to preserve this precious pigment. To achieve these objectives, a combination of µXRF, Cl and S K-edge µXANES and Hg L3 edge µXANES in HERFD mode is crucial.

Identifier
DOI https://doi.org/10.15151/ESRF-ES-756167862
Metadata Access https://icatplus.esrf.fr/oaipmh/request?verb=GetRecord&metadataPrefix=oai_datacite&identifier=oai:icatplus.esrf.fr:inv/756167862
Provenance
Creator Hiram CASTILLO; Francesco CARUSO ORCID logo; Edgar Eduardo VILLALOBOS PORTILLO ORCID logo; Marine COTTE (ORCID: 0000-0002-4949-588X); Maite MAGUREGUI ORCID logo; Francesco GIANNICI (ORCID: 0000-0003-3086-956X)
Publisher ESRF (European Synchrotron Radiation Facility)
Publication Year 2025
Rights CC-BY-4.0; https://creativecommons.org/licenses/by/4.0
OpenAccess true
Representation
Resource Type Data from large facility measurement; Collection
Discipline Particles, Nuclei and Fields